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From secondary ion mass spectrometry (SIMS) conducted for the rod with a diameter of 20mm (Supplementary Fig. 1), it is clear that the dendrites are Ti rich, Cu and Co lean. The Be signal in Ti is very week, suggesting that only a very small amount of Be is dissolved in Ti, a phenomenon commonly observed in Be containing BMGCs17,20.

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Molar ratios of Ga3+/Ga+ are 0.16/0.84 at 2V and 0.52/0.48 at 2V in the 2nd sweep cycle and 0.19/0.81 at 2V, 0.28/0.71 at 1.3V and 0.50/0.50 at 2V in the 3rd sweep cycle, as calculated by peak fitting analysis. (d) Near Fermi edge spectra of a GaOx film: pristine (black), HRS (at +2V) (red) and LRS (at 2V) (blue). The density of states near the top of the valence band is variable by negative or positive biasing.

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